Hi Daniel
I have done that the entire Litoral from Santos up to Natal, and crossed several rivers with barcos etc. just at some points e.e. Porto Seguro, you have to get back to the 101. Breathtaking small unpaved (enduro) roads from Aracaju until Recife.
But it is worth also to leave Palmares 100 Km south of Recife for Caruaru, the largest feira de artesana in Brasil, and drive back to Recife on a brand new 4 lane highway.
I have much more info on that, and will be back for a Brasil roundtrip on my bike in Sept .
rgds
Rainer
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