I've not ridden the CRF much, but have 2 TTRs, one with a 315cc big bore and another with a 350. I love them and have done a lot of miles on them. In my opinion the Yamaha suspension is really good, especially for it's age - effectively unchanged from 1993 and is easy to adjust for load carrying. The standard 250 engine pulls well and is reliable. Starter sprag clutches suffer from irregular oil changes on older bikes. (Easy to change, check parts prices on www.totallyttrs.com) Carbs are prone to blockages on older bikes from lack of use, old fuel residues etc. Rear subframe is a bit weak for load carrying but a bit of simple triangulation bracing is easy to do. There is masses of information on YAMAHA TTR250 TRAIL and OFFROAD MOTORCYCLE FAQ and a very supportive and informative forum at https://www.ttr250.activeboard.com/
I think the CRF is a bit overweight and poorly suspended in comparison, but you might find it more ergonomically pleasant, and the frame is more substantial for luggage. Both bikes should manage 70mph with the right gearing but neither will be pleasant without a screen of some kind. The TTR is a much better trail bike IMHO, but travel bike... being honest, that's a more difficult call. I would, and many others have. See if you can at least sit on one, and enjoy the decision making process. It's part of the fun!
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