If you're interested primarily in riding/nature/scenery, head down to the High Tatras in Slovakia, maybe take in Zakopanie on the way. (My bucket list has Morskie Oko lake on it, YMMV.)
If you're interested in fascinating Eastern Block stuff, head to Lviv. Then maybe play around in Ukrainian Carpathia, see how far you can get before you have to turn back.
Krakow is worth a stopover and on the way in any case.
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